Spin-resolved ARPES

Spin-resolved ARPES

Spin-resolved ARPES extends conventional angle-resolved photoemission spectroscopy by measuring not only the energy and momentum of photoemitted electrons, but also their spin polarization, thereby providing direct access to the spin-dependent electronic structure of a material. This is achieved by directing photoelectrons into a spin polarimeter, where spin-dependent scattering processes reveal the orientation of the electron spin along one or more axes.

By combining momentum, energy, and spin information, spin-resolved ARPES can uncover the spin textures associated with spin-orbit coupling, broken inversion symmetry, magnetic order, and spin-orbital entanglement. The technique has been essential for establishing the helical spin structure of topological surface states, quantifying Rashba and related spin splittings, and revealing subtler forms of entanglement between spin, orbital, and band degrees of freedom in complex quantum materials.

Our group uses spin-resolved ARPES to investigate how spin and orbital character are intertwined in topological, correlated, and spin-orbit-coupled materials, and to connect these observations directly to the underlying symmetry and many-body structure of their electronic states.

Publications

Constraints on the two-dimensional pseudo-spin 1/2 Mott insulator description of Sr2IrO4

B. Zwartsenberg, R. P. Day, E. Razzoli, M. Michiardi, M.X. Na, G. Zhang, J.D. Denlinger, I. Vobornik, C. Bigi, B.J. Kim, I.S. Elfimov, E. Pavarini, A. Damascelli. Phys. Rev. B 105(24), 245130 (2022).

Influence of Spin-Orbit Coupling in Iron-Based Superconductors

R.P. Day, G. Levy, M. Michiardi, B. Zwartsenberg, M. Zonno, F. Ji, E. Razzoli, F. Boschini, S. Chi, R. Liang, P.K. Das, I. Vobornik, J. Fujii, W.N. Hardy, D.A. Bonn, I.S. Elfimov, A. Damascelli. Phys. Rev. Lett. 121(7), 76401 (2018).

Spin-Orbital Entanglement and the Breakdown of Singlets and Triplets in Sr2RuO4 Revealed by Spin- and Angle-Resolved Photoemission Spectroscopy

C.N. Veenstra, Z.-H. Zhu, M. Raichle, B.M. Ludbrook, A. Nicolaou, B. Slomski, G. Landolt, S. Kittaka, Y. Maeno, J.H. Dil, I.S. Elfimov, M.W. Haverkort, A. Damascelli. Phys. Rev. Lett. 112, 127002 (2014).

Photoelectron Spin-Polarization Control in the Topological Insulator Bi2Se3

Z. Zhu, C.N. Veenstra, S. Zhdanovich, M.P. Schneider, T. Okuda, K. Miyamoto, S. Zhu, H. Namatame, M. Taniguchi, M.W. Haverkort, I.S. Elfimov, A. Damascelli. Phys. Rev. Lett. 112, 76802 (2014).
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